Total Recommendations: 1
If you liked
Gokukoku no Brynhildr
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...then you might like
Shuumatsu Nani Shitemasu ka? Isogashii desu ka? Sukutte Moratte Ii desu ka?
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Both animes share a similar sadly dark feeling where the MC is the only person who really cares and tries to save a bunch of 'magical' girls in trouble AND he also develops a romantic relationship with one of the girls.