If you liked
Code Geass: Hangyaku no Lelouch
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...then you might like
Psycho-Pass
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Both have the same premise of bringing down a corrupt government and questions whether it's better to bring it down from outside or work from within to change it. Both have psychological and ideological themes that will have you thinking about for a long time after you've finished watching and make a point to confuse you about whether the ends or the means are correct (Code Geass is more emphatic on this) and that not everything is black and white (well duh): you'll have to reflect and decide on your own about what you think is right. As for differences, Psycho-Pass lacks the super-powered piloted robots in Code Geass but makes up for it using "Dominators" (huge badass guns, basically). Psycho-Pass surpasses CG in terms of artwork and animation by far, however. PP also doesn't mess up its characters arcs like Code Geass (although CG's first season is better than the second in terms of this).