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If you liked Chuunibyou demo Koi ga Shitai! add

...then you might like Hana to Alice: Satsujin Jiken add

Okay Chunibyo is much more flashy and crazy than Hana to Alice, but it has that theme of new friendships and helping someone who is not all there mentally recover by solving a mystery. But most important of all the characters in Hana to Alice are definitely Chuunibyou.

If you liked FLCL add

...then you might like Arakawa Under the Bridge x Bridge add

FLCL deals with a group of crazy characters and one of them is homeless as well, I think.