If you liked
Kokoro Connect
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...then you might like
Seishun Buta Yarou wa Bunny Girl Senpai no Yume wo Minai
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Both are high school anime focusing on a main character who has the desire to help those around him, especially his closest friends. For every arc is a new supernatural event that occurs due to a problem that one or more of the characters is experiencing, yet has been hiding from the others. With this supernatural event the character or characters involved cannot hide themselves for very long, otherwise they'd suffer very terrible consequences that could harm not only themselves but those around him/her.
If you liked
Sakura-sou no Pet na Kanojo
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...then you might like
Yahari Ore no Seishun Love Comedy wa Machigatteiru.
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Both Sakurasou and Oregairu delve into the problems and difficulties high school students will face. While Oregairu focuses mostly on the social problems and what happens presently, Sakurasou focuses a lot more on what each character will do an choose for their future. Overall, both are unique and entertaining romantic comedies.
If you liked
Fullmetal Alchemist: Brotherhood
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...then you might like
Mahou Shoujo Madoka★Magica
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Both animes take on a similar trope; in which to obtain something, an equal thing force must be sacrificed. Definitely recommend anyone who has watched FMAB to watch this series. Do not let the title fool you, this series is much darker than you may expect.