Kiwamete Gouman Taru Akuyaku Kizoku no Shogyou
The Deeds of an Extremely Arrogant Villainous Noble

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The story has a protagonist in a Polyamory with romantic development in Fantasy/Isekai. Includes 'Polygamy with romantic development', 'Multiple Lovers/Multiple Partners in an open romantic relationship', or an open romantic relationship with a harem. Also True Harem, Harem Ending, Harem-seeking, Hard-Working, Devoted, Couple Growth, First-time Intercourse, Marriage tag.

(PART 1) https://myanimelist.net/stacks/36913

Additional (currently no MyAnimeList page):
-(Manhwa) Trapped in a Hentai Game Academy / Trapped in the Academy's Eroge (currently 105 chapters)
-(Manhwa) The Main Heroines are Trying to Kill Me (Unless read WN)
-(Manhwa) Fated to Be Loved by Villains (Currently confirm)(Unless read WN)
-(Chinese Manhua) Yao Shen Ji / Tales of Demons and Gods (currently 478 chapters)
-(Light Novel) Bannousugiru Souzou Skill de Isekai wo Shitataka ni Ikiru! / Chronicles of a Creative Different World Reincarnation (completed v05)
-(Manga) Ii Gomibun da na, Ore ni Kureyo / What Good Social Status You Have. Give It to Me. (Unless read WN)
-(Manga) Isekai de Kuchizuke wo! Tensei Sekai wa Unmei no Hito de Michiteiru (Currently confirm)
-(Manga) Maou wo Taoshita Ore ni Matteita no wa, Sewazuki na Yome to no Ichaicha Renkin Seikatsu datta / After Defeating the Demon King, What Awaited Me Was a Lovey-Dovey Alchemical Life With a Caring Wife (currently 27 chapters)
-(Manga) Doryoku wa Ore wo Uragirenai / Hard Work Will Never Betray Me (Currently confirm)(Unless read LN)
-(Manga) Potion Kouji ni Sasensareta Ore Renkinjutsushi, Bishoujo ni Rachisare Ikoku de Itsunomanika Eiyuu ni naru / I, Who Was Demoted to a Potion Factory, Was Kidnapped by an Elf and Became an Alchemist in a Desert Country (Currently confirm)(Unless read WN)
-(Manga) Kiss kara Hajimaru Isekai Harem ~Ipputasai no Sekai ni Tensei shita node Kami ga Kimeta Unmei no Hito wo Sagashimasu~ (Currently confirm)
-(Manga) Millimos Saga: Battei Ouji no Tensei Senki (Currently confirm)(Unless read WN)
-(Manga) Game Sekai Tensei "Dunkatsu" / Reincarnated in the game world "Dungeon Activity" (Currently confirm)(Unless read WN)

Additional:
51- Akumade Taidana Akuyaku Kizoku / The Slothful Villainous Noble (Currently confirm)(Unless read WN)
52- Surviving in a Romance Fantasy Novel (Currently confirm)(Unless read WN)
53-
54-
A 'Part 3' will be created if this list goes up to 60.

Protagonist is transmigrated/reincarnated into an Book/Novel world. Also Transmigration/Reincarnation. Includes Comic/Manga World, TV Show/TV Drama World.

(PART 1) https://myanimelist.net/stacks/37920
(PART 4) https://myanimelist.net/stacks/56037