 If you liked
Totsukuni no Shoujo
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 ...then you might like
Akuma-san to Outa
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Akuma-san to Outa is a lot sillier than Siúil a Rún, but both are bittersweet stories of monstrous caretakers and and the children that adore them. Hetappi and Shiva are both bright, cheerful children that have been abandoned and punished by their religious society. They are both taken care of by creatures deemed evil by humanity, but are quickly established as loving and selfless caretakers. Without getting into spoilers, there's some darker thematic similarities between both series (while again Akuma-san to Outa is a lot goofier and frank in their presentation.)