If you liked
Kimi wa Pet
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...then you might like
Sakuranbo Syndrome - Cupid no Itazura II
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Both series focuses on relationships but in rather unorthodox circumstances. In essence, their story connects characters through friendship and romance. The main male protagonist also has similar personalities - caring, compassionate, and helpful. The female protagonist on the other hand has more of a childish personality but does show their mature side as the series progresses. Both series are also known for their drama involving other characters that gets involved in their relationships; recommended for fans looking for a mature seinen or shoujo.