 If you liked
Mai-HiME
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 ...then you might like
Uta∽Kata
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Both are mahou shoujo shows that start out happy, but then become very dark and sometimes brutal. Both show the gradual mental breakdown of the protagonists.
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Recommended by _mahoushoujos_
Both are magical girl stories that start off cute but get more darker as time goes by.
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Recommended by Disapeared_Ghost