 If you liked
Shuffle!
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 ...then you might like
Negima!?
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They both are harem/ magical anime, for one. Also, they both are just brilliant shows. Sure, Negima may center around a magical classroom, but Shuffle expands from the classroom into showing how this magical girls interact with the world. Negima had robots, ninjas, vampires, wizards, ghosts, etc. Shuffle has angels and demons, a kind of step up. So i definately reccomend Shuffle for Negima lovers.