 If you liked
Mahou Shoujo Lyrical Nanoha
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 ...then you might like
Uta∽Kata
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They're both Mahou Shoujo shows but there's a thing that seperates them from other Mahou Shoujo shows. Both are pretty cliché at first sight but after a few episodes a darker storyline will appear. Both shows have drama and pretty serious issues, not suitable for the age group of many other Mahou Shoujo shows.
Both are darker mahou shoujo shows with a little bit of fan service. Neither one is actually geared at little girls and are not part of the shoujo genre, but rather closer to seinen. Both shows also explore a relationship between two magical girls in particular rather than a huge group.