 If you liked
Suzumiya Haruhi no Shoushitsu
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 ...then you might like
Arakawa Under the Bridge
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To be honest they're both kinda wack, but that's what makes both of these anime so unique. Both anime take a normal guy, the protagonist, and put him with a bunch of crazy people! The animation in both anime is very crisp, and the mood is light. Plot and character development aren't major in either anime, but character interaction is. The stories both flow, and the voice actors do great jobs. Mostly comedy but also some romance and a tiny little bit of action. They're both really unique and spontaneous based anime, so if you watch for comedy then you're sure to enjoy!