 If you liked
Suzumiya Haruhi no Shoushitsu
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 ...then you might like
Mahou Shoujo Madoka★Magica Movie 2: Eien no Monogatari
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Shifting focus from a multiple character cast to maily two characters? Check.
A further exploration of their personal experiences and the consequences of said experiences? Check.
A further exploration of the connection these two characters have and how it affects their own lives & the existence of those around them? Check.
Gorgeous visuals and quality fluid animation? Check.
Fantastic cinematography and great directing? Check.
A sequel that offers closure, yet leaves enough open for a possible future sequel? Check.
Cute girls suffering? Check (let's be real, we can't deny it's true).
Beautiful soundtrack? Check.
[Sort of spoiler] Time-travel done right with a proper explanation of its rules and how it functions? Check.