 If you liked
Casshern Sins
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 ...then you might like
Dororo
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Both casshern and hyakkimaru find killing and destroying as their only reason for living but they soon gain the heart to love someone after meeting a small child(ringo and dororo). So if u love animez where an innocent smile can change a heartless MC, u'll probably like these two.
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Recommended by yabuki-kun
Both characters starts off from a position, in which they don't have direction in their existence, or meaning in it. Their drive to understand themselves is the one that keeps them going, and along their ways, they learn to be more humane and empathetic with each encounter from someone in this life - be it pain, or happiness, everyone leaves impression in them.