 If you liked
Koukaku Kidoutai
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 ...then you might like
Vivy: Fluorite Eye's Song
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Both stories revolve around a cybernetic being that involves deep introspection, character development, and scenes of combat. And both explore the theme of what happens when AI life has a soul of it's own? And they are both easily very good masterpiece-level anime. I definitely recommend both.
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Recommended by Sara_Isayama
Both protagonists are AI that have to fight to save something. They have the same dark vibe, and a lot of good action scenes. They both analyze the topic of "Humans vs AI"