 If you liked
Serial Experiments Lain
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 ...then you might like
Psycho-Pass
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Both have technological advancement with dark theme and character with twisted belief or rather unorthodox way of thinking. both have lots of questions about the existence of anything in this world.
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Recommended by kashimkurz
both are intense dramas of the cyberpunk, psychological, and sci-fi genre, and both focus on cryptic mysteries and details related to their plots.
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Recommended by NintensityCrowds
Both are cyberpunk themed stories that focus around the concept of technolgy being used for evil purposes and a girl with an innocence to them getting caught up in the strange events.
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Recommended by Disapeared_Ghost