 If you liked
Kuro Ai: Hitoyozumakan Inkou Rannyuuroku
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 ...then you might like
Taimanin Asagi
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Same director, the KING of Hentai in my mind. Both have gorgeous animation, both are quite hard core, both have tentacles, both are along the occult.
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Recommended by DolorDecorus
They have fast-paced, skaky-camera, and very nice, animation. Both have villains and hardcore scenes.
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Recommended by herlegacys