If you liked
Gankutsuou
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...then you might like
Code Geass: Hangyaku no Lelouch
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Both involve deep, brilliant, complex storylines which have you sat on the edge of your seat all the way through. Masterpieces, involving lots of character development and twists and turns in the story. Although they are different genres, both have high emotional content and have the ever advancing (with every episode) sense of doom.
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Recommended by sugarplumfairy
Both are very story-driven, with lots of suspense and twists. Both also have numerous aristocratic main characters.
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Recommended by RoboticEarthling
Both animes revolve around a character being betrayed and them seeking vengeance however, they differ when it comes down to the method where Code Geass involves balls to the wall action Gankutsuo uses more subtle means as it follows Alexandre Dumas' The Count of Monte Cristo with a few changes(by a few mean a shit ton like it's in the future and mechs for some reason).