 If you liked
Darker than Black: Kuro no Keiyakusha
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 ...then you might like
Un-Go
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Even though the plots are different when one is about being an assassin and one a detective but they gives of the same feeling.
They both deal with supernatural beings and the main characters are in confusion of betrayal, also they lost someone dear to them. Both anime also have human-like beings (Doll/AI)
Both anime contain mystery and investigation, with gloomy and dark aura. But darker than black contains actions which Un-GO doesn't since it focuses on the mystery part.
Watching Darker than black reminds me of Un-GO.
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Recommended by Queen_Vania