 If you liked
RahXephon
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 ...then you might like
The SoulTaker: Tamashii-gari
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Early 2000's shows with very attractive character designs and just interesting visuals in general. Both have basically nonsensical (sometimes laughable) storylines, with weird sibling connections, female harems, mecha-esque creatures figthing aliens and some existential monologues (usually about being an alien or not).
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Recommended by DsMasterBR