 If you liked
Code Geass: Hangyaku no Lelouch
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 ...then you might like
Yu☆Gi☆Oh! VRAINS
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Both have genius level intellect main characters who rebel against the status quo due to the tragic and traumatic past. Both have nice character designs with clean art styles & lovable characters.
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Recommended by JVskunkape
Characters with alter egos set out in their pursuit of vengeance aided by a mysterious companion with special powers.
Note that AI and Suzaku shares the same Seiyuu making this series another CG comparison.
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Recommended by WingZeroRequiem