 If you liked
Brigadoon: Marin to Melan
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 ...then you might like
Mahoutsukai no Yome
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The creator of the Ancient Magus Bride stated in Volume 1 of her manga that Brigadoon was an influence on her. And this should be clear just by looking at the shows. Both are about a girl with no parents who experiences tragedy in their lives, while forming a bond with a powerful nonhuman male creature that protects them. Both are about the love between the girl and her protector and appear to be shojou "girl's shows" at first but actually feature violent and bloody battles, with human characters dying.
Both shows are really unlike anything out there, and highly recommended.
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Recommended by BandDog_Onymou