 If you liked
Psycho-Pass
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 ...then you might like
Btooom!
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Anime that have dark themes and deal with killing others in a very distant, cold, calculated way though both main characters have to deal with it emotionally it themselves. Both characters face dark and twisted opponents who show the darker side of human nature, especially when the normal social restraints are removed either from the lack of civilization or a broken criminal justice system. The animes are both violent and graphic.
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Recommended by yngtadpole