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If you liked Gankutsuou add

...then you might like Masamune-kun no Revenge add

Both of these are tales of revenge (Gankutsuou being based off the archetypal revenge plot from The Count of Monte Cristo). Gankutsuo is certainly heavier than Masamune-kun's high school antics, but I think you will enjoy watching the vindictive machinations of a character seeking to deal punishment for past wrongs.

If you liked Nisekoi add

...then you might like Yamada-kun to 7-nin no Majo add

Both of these shows are high school harems with a protagonist who has a heart of gold (granted Yamada is bit rougher around the edges).